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Froid par sorption à base d'eau à très basse température grâce à un aluminophosphate poreux de type zéolite peu coûteux.

Ultralow-temperature-driven water-based sorption refrigeration enabled by low-cost zeolite-like porous aluminophosphate.

Auteurs : LIU Z., XU J., XU M., HUANG C., WANG R., LI T., HUAI X.

Type d'article : Article de périodique

Résumé

Thermally driven water-based sorption refrigeration is considered a promising strategy to realize near-zero-carbon cooling applications by addressing the urgent global climate challenge caused by conventional chlorofluorocarbon (CFC) refrigerants. However, developing cost-effective and high-performance water-sorption porous materials driven by low-temperature thermal energy is still a significant challenge. Here, we propose a zeolite-like aluminophosphate with SFO topology (EMM-8) for water-sorption-driven refrigeration. The EMM-8 is characterized by 12-membered ring channels with large accessible pore volume and exhibits high water uptake of 0.28 g·g−1 at P/P0 = 0.2, low-temperature regeneration of 65 °C, fast adsorption kinetics, remarkable hydrothermal stability, and scalable fabrication. Importantly, the water-sorption-based chiller with EMM-8 shows the potential of achieving a record coefficient of performance (COP) of 0.85 at an ultralow-driven temperature of 63 °C. The working performance makes EMM-8 a practical alternative to realize high-efficient ultra-low-temperature-driven refrigeration.

Détails

  • Titre original : Ultralow-temperature-driven water-based sorption refrigeration enabled by low-cost zeolite-like porous aluminophosphate.
  • Identifiant de la fiche : 30029226
  • Langues : Anglais
  • Sujet : Technologie
  • Source : Nature Communications - 13
  • Éditeurs : Springer Nature
  • Date d'édition : 11/01/2022
  • DOI : http://dx.doi.org/10.1038/s41467-021-27883-4

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